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Only a portion of this set is Gold Signature.
It is a complete set of 100 cards, 34 of which are Gold Signature cards.
Below is listed the cards that ARE gold signature.
Gold Signature List
3 - Bishop
4 - Cannonball
15 - Havok
17 - Random
26 - Douglock
30 - Chamber
31 - Husk
34 - Mondo
36 - Skin
38 - White Queen
43 - Deadbolt
49 - Tusk
51 - Deadpool
52- Kane
56 - Maverick
57 - Raza
58 - Albert
64 - Emplate
65 - Gladiator
67 - Lady Deathstrike
68 - Legion
73 - Orphan Maker
75 - Sentinels
76 - Silver Samurai
77 - Spiral
78 - Stryfe
82 - Weapon X
83 - Department H
91 - Colossus as Count Vampire
92 - Cyclops as the King
95 - Professor X as the Wizard of X
96 - Psylocke as the French Maid
97 - Roger as the Vampiress
98 - Storm as the Witch